本文主要研究内容
作者（2019）在《Conversion of CO2 to ethanol by using a metal-organic framework catalyst》一文中研究指出：With the development of CO2 capture technology, CO2 can become an attractive C1 resource for synthesizing commodity chemicals. For example, direct conversion of CO2 to ethanol is of interest, but this process is also quite challenging, because it requires both the formation of one C–C bond and the retention of one C–O bond [1]. A combination of dual active sites, one for methanol formation and one for C–C coupling has been widely investigated for such a conversion, but an unbalanced rate in the two steps frequently leads to the formation of either methanol or long-chain hydrocarbons [2].
Abstract
With the development of CO2 capture technology, CO2 can become an attractive C1 resource for synthesizing commodity chemicals. For example, direct conversion of CO2 to ethanol is of interest, but this process is also quite challenging, because it requires both the formation of one C–C bond and the retention of one C–O bond [1]. A combination of dual active sites, one for methanol formation and one for C–C coupling has been widely investigated for such a conversion, but an unbalanced rate in the two steps frequently leads to the formation of either methanol or long-chain hydrocarbons [2].
论文参考文献
[1].Pd nanoparticles immobilized on MIL-53(Al) as highly e ective bifunctional catalysts for oxidation of liquid methanol to methyl formate[J]. Jian-Fang Liu,Jin-Cheng Mu,Rong-Xian Qin,Sheng-Fu Ji. Petroleum Science.2019(04)[2].Synthesis of graphene-supported monodisperse Au Pd bimetallic nanoparticles for electrochemical oxidation of methanol[J]. 肖红君,申承民,时雪钊,杨苏东,田园,林少雄,高鸿钧. Chinese Physics B.2015(07)[3].Dynamic modeling of a H2O-permselective membrane reactor to enhance methanol synthesis from syngas considering catalyst deactivation[J]. M.Farsi,A.Jahanmiri. Journal of Natural Gas Chemistry.2012(04)[4].Simultaneous production and utilization of methanol for methyl formate synthesis in a looped heat exchanger reactor configuration[J]. A.Goosheneshin,R.Maleki,D.Iranshahi,M.R.Rahimpour,A.Jahanmiri. Journal of Natural Gas Chemistry.2012(06)[5].Pd-gate MOS sensor for detection of methanol and propanol[J]. Preeti Pandey,J. K. Srivastava,V. N. Mishra,R. Dwivedi. Journal of Natural Gas Chemistry.2011(02)[6].Competition between Imported and Domestic Methanol[J]. Liu Zhiguang,Deputy Chief Engineer of China National Petroleum and Chemical Planning Institute. China Chemical Reporter.2010(13)[7].Promoting effect of polyoxyethylene octylphenol ether on Cu/ZnO catalysts for low-temperature methanol synthesis[J]. Ling Liu,Tiansheng Zhao,Qingxiang Ma,Yufang Shen Key Laboratory of Energy Resources & Chemical Engineering of Ningxia,Ministry-Province Co-Cultivated State Key Laboratory Base,Ningxia University,Yinchuan 750021,Ningxia,China. Journal of Natural Gas Chemistry.2009(03)[8].Solvent effects on Pt-Ru/C catalyst for methanol electro-oxidation[J]. Jinwei Chen,Chunping Jiang,Hui Lu,Lan Feng,Xin Yang,Liangqiong Li,Ruilin Wang College of Materials Science and Engineering,Sichuan University,Chengdu 610065,Sichuan,China. Journal of Natural Gas Chemistry.2009(03)[9].Coal-to-Olefins Conference 2009[J]. China Chemical Reporter.2009(19)[10].Donghua Energy Kicks off 1.2 Million T/A Methanol Project[J]. China Chemical Reporter.2009(15)
论文详细介绍
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：Conversion of CO2 to ethanol by using a metal-organic framework catalyst论文
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